I would go back in time to the 1980s, and implement a plan to move the entire Storrs campus to Hartford by 2010. Investing billions over the last few decades into a campus in the woods of eastern Connecticut that the locals do not even want there while also investing billions into a small city like Hartford was wasted investment dollars. If UConn was in the state capital, 1) it would be higher ranked academically, 2) it would be a more desirable conference partner, 3) Hartford would be a much nicer city, and 4) the state of Connecticut would have saved billions over the last 35 years.
I have been told that this was actually discussed in the late 80's and early 90's among state legislators, but after some rough budget cycles, the will to make a big change never developed.